Physical Review Letters · 2018 · 203 citations · 45 references
Natural SciencesPhysicsCondensed Matter PhysicsPhotonicsSolid State PhysicsElectronic Band StructureElectronic Structure Of SolidsOptical Properties Of SolidsTopological MaterialsTopological Phases Of MatterUltrafast OpticsBand GapHarmonic GenerationHigh-harmonic GenerationHigh-order Harmonic GenerationPeriodic StructureStrong-field Laser-matter InteractionTime-dependent Density Functional TheoryTopological Edge States
High-harmonic generation in the two topological phases of a finite, one-dimensional, periodic structure is investigated using a self-consistent time-dependent density functional theory approach. For harmonic photon energies smaller than the band gap, the harmonic yield is found to differ by up to 14 orders of magnitude for the two topological phases. This giant topological effect is explained by the degree of destructive interference in the harmonic emission of all valence-band (and edge-state) electrons, which strongly depends on whether or not topological edge states are present. The combination of strong-field laser physics with topological condensed matter opens up new possibilities to electronically control strong-field-based light or particle sources or-conversely-to steer by all optical means topological electronics.
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