Quantized circular photogalvanic effect in Weyl semimetals

Fernando de Juan, Adolfo G. Grushin, Takahiro Morimoto, Joel E. Moore

Nature Communications · 2017 · 701 citations · 58 references

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Concepts

TL;DR

The circular photogalvanic effect (CPGE) is a photocurrent component that reverses with the sense of circular polarization and has been consistently observed in non‑centrosymmetric systems, though its magnitude depends on material‑specific details. The CPGE directly probes the topological charge of Weyl points, and disorder or additional band contributions can be negligible over a broad frequency range, leading to an effectively quantized response. In Weyl semimetals such as SrSi$_2$ and three‑dimensional Rashba materials like doped Te, the injection CPGE is quantized in terms of fundamental constants with no material‑dependent parameters, and its sizable magnitude allows direct detection of the monopole charge using current techniques.

Abstract

The circular photogalvanic effect (CPGE) is the part of a photocurrent that switches depending on the sense of circular polarization of the incident light. It has been consistently observed in systems without inversion symmetry and depends on non-universal material details. Here we find that in a class of Weyl semimetals (e.g. SrSi$_2$) and three-dimensional Rashba materials (e.g. doped Te) without inversion and mirror symmetries, the injection contribution to the CPGE trace is effectively quantized in terms of the fundamental constants $e, h, c$ and $\epsilon_0$ with no material-dependent parameters. This is so because the CPGE directly measures the topological charge of Weyl points, and non-quantized corrections from disorder and additional bands can be small over a significant range of incident frequencies. Moreover, the magnitude of the CPGE induced by a Weyl node is relatively large, which enables the direct detection of the monopole charge with current techniques.

References

58