Nature Communications · 2017 · 701 citations · 58 references
Natural SciencesMaterials SciencePhysicsCondensed Matter PhysicsElectronic MaterialsQuantum MechanicsElectronic Band StructureQuantum OptoelectronicsTopological MaterialsTopological Phases Of MatterCircular PolarizationDirac SemimetalsFundamental Physical ConstantsInversion SymmetrySymmetriesTopological Band StructureTopological SemimetalsWeyl Semimetals
The circular photogalvanic effect (CPGE) is a photocurrent component that reverses with the sense of circular polarization and has been consistently observed in non‑centrosymmetric systems, though its magnitude depends on material‑specific details. The CPGE directly probes the topological charge of Weyl points, and disorder or additional band contributions can be negligible over a broad frequency range, leading to an effectively quantized response. In Weyl semimetals such as SrSi$_2$ and three‑dimensional Rashba materials like doped Te, the injection CPGE is quantized in terms of fundamental constants with no material‑dependent parameters, and its sizable magnitude allows direct detection of the monopole charge using current techniques.
The circular photogalvanic effect (CPGE) is the part of a photocurrent that switches depending on the sense of circular polarization of the incident light. It has been consistently observed in systems without inversion symmetry and depends on non-universal material details. Here we find that in a class of Weyl semimetals (e.g. SrSi$_2$) and three-dimensional Rashba materials (e.g. doped Te) without inversion and mirror symmetries, the injection contribution to the CPGE trace is effectively quantized in terms of the fundamental constants $e, h, c$ and $\epsilon_0$ with no material-dependent parameters. This is so because the CPGE directly measures the topological charge of Weyl points, and non-quantized corrections from disorder and additional bands can be small over a significant range of incident frequencies. Moreover, the magnitude of the CPGE induced by a Weyl node is relatively large, which enables the direct detection of the monopole charge with current techniques.
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