A Metal–Insulator Transition of the Buried MnO₂ Monolayer in Complex Oxide Heterostructure

Abstract

A novel artificially created MnO₂ monolayer system is demonstrated in atomically controlled epitaxial perovskite heterostructures. With careful design of different electrostatic boundary conditions, a magnetic transition as well as a metal-insulator transition of the MnO₂ monolayer is unveiled, providing a fundamental understanding of dimensionality-confined strongly correlated electron systems and a direction to design new electronic devices.