Universal nonlinear scattering in ultra-high Q whispering gallery-mode resonators

Abstract

Universal nonlinear scattering processes such as Brillouin, Raman, and Kerr effects are fundamental light-matter interactions of particular theoretical and experimental importance. They originate from the interaction of a laser field with an optical medium at the lattice, molecular, and electronic scale, respectively. These nonlinear effects are generally observed and analyzed separately, because they do not often occur concomitantly. In this article, we report the simultaneous excitation of these three fundamental interactions in mm-size ultra-high Q whispering gallery mode resonators under continuous wave pumping. Universal nonlinear scattering is demonstrated in barium fluoride and strontium fluoride, separately. We further propose a unified theory based on a spatiotemporal formalism for the understanding of this phenomenology.