Journal of the Atmospheric Sciences · 1977 · 3.8K citations · 0 references
Natural SciencesEarth SciencesMeteorologyAir PollutionAtmospheric ScienceCloud PhysicsAerosol-cloud InteractionsAtmospheric OpticsCloud Optical PropertiesCloud ProcessesCloud PropertiesCloud StructureAerosol Optical ThicknessAlbedoCloud AbsorptionCloud ReflectanceCloud Shortwave Optical PropertiesOptical Absorption CoefficientShortwave AlbedoThickness-dependent Optical Properties
By increasing droplet concentration and thereby the optical thickness of a cloud, pollution acts to increase the reflectance (albedo) of clouds; by increasing the absorption coefficient it acts to decrease the reflectance. Calculations suggest that the former effect (brightening of the clouds in reflection, hence climatically a cooling effect) dominates for thin to moderately thick clouds, whereas for sufficiently thick clouds the latter effect (climatically a warming effect) can become dominant.