Publication | Closed Access
A Complete Catalytic Cycle for Supramolecular Methanol‐to‐Olefins Conversion by Linking Theory with Experiment
268
Citations
33
References
2008
Year
Chemical EngineeringSupramolecular Methanol‐to‐olefins ConversionEngineeringAlkene MetathesisIndustrial CatalysisComplete Catalytic CycleMethanolCatalytic SynthesisOrganic ChemistryMethylbenzene RingCatalysisOrganometallic CatalysisChemistryCatalytic CycleHomogeneous CatalysisMolecular CatalysisLe TourBiomolecular Engineering
Le Tour de MTO: A complete working catalytic cycle for the conversion of methanol to olefins in HZSM-5 is reported in full consistency with both experimental and theoretical observations. This particular route includes carbon-atom scrambling into a methylbenzene ring, NMR-observed cationic intermediates, and the production of isobutene.
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