GAS ABSORPTION INTO WAVY AND TURBULENT FALLING LIQUID FILMS IN A WETTED-WALL COLUMN

Abstract

Experiments are conducted for gas absorption in a long wetted-wall column. Liquid-side mass transfer coefficients are measured for absorption of CO2 and O2 into falling water films on the outside of a stainless steel pipe 2.72 cm OD and 183 cm absorption length. The liquid film Reynolds number ranges from 129 to 10500 which encompasses the wavy-laminar, wavy-transition and turbulent flow regimes. The experimental data are correlated by a dimensionless equation of the form kt = (ktD) (v2/g) 1/3 = a-Rep-Sc1/2. The correlation is well supported by a viscosity-damped turbulence model at the gas-liquid interface which tends to confirm that viscosity is probably the major mechanism causing eddy damping and not surface tension as proposed by Levich and Davies. The form of the above correlation also represents previous experimental work at different temperatures and for different gases quite well.