Physical Review Letters · 2013 · 117 citations · 41 references
Natural SciencesPhysicsColloid ScienceCondensed Matter PhysicsSolid State PhysicsCondensed Matter TheoryCritical PhenomenaDisordered SystemsPhase EquilibriaPhase TransitionsStates Of MatterColloidal Phase TransitionsIntermediate Phase FormationKosterlitz-thouless TransitionMelting BehaviorPhase Behavior Of ColloidsQuenched DisorderQuenched PhasesTwo-dimensional Melting
We study the influence of quenched disorder on the two-dimensional melting behavior of superparamagnetic colloidal particles, using both video microscopy and computer simulations of repulsive parallel dipoles. Quenched disorder is introduced by pinning a fraction of the particles to an underlying substrate. We confirm the occurrence of the Kosterlitz-Thouless-Halperin-Nelson-Young scenario and observe an intermediate hexatic phase. While the fluid-hexatic transition remains largely unaffected by disorder, the hexatic-solid transition shifts to lower temperatures with increasing disorder. This results in a significantly broadened stability range of the hexatic phase. In addition, we observe spatiotemporal critical(like) fluctuations, which are consistent with the continuous character of the phase transitions. Characteristics of first-order transitions are not observed.
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