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Vibrational excitations of a one-dimensional electron-phonon system in strong coupling
35
Citations
6
References
1978
Year
Quantum DynamicQuantum ScienceVibronic InteractionPhonon SpectrumEngineeringPhysicsOptical PropertiesStrong CouplingApplied PhysicsCondensed Matter PhysicsQuantum MaterialsPhonon Frequency SpectrumExcitation Energy TransferPhononQuantum SolidNonlinear ResonanceModified Phonon Spectrum
We consider an electron interacting with optical phonons through the deformation potential in one dimension. We calculate the energy spectrum of such a system to one order in $\frac{1}{{\ensuremath{\alpha}}^{2}}$ beyond the strong-coupling limit. We calculate the self-energy, effective mass and modified phonon spectrum to this order. The modified phonon spectrum is determined by the solution of a homogeneous linear integral equation. We are able to solve this integral equation in closed form for the odd-parity phonon modes. The result is a frequency spectrum ${\ensuremath{\Omega}}_{n}={\ensuremath{\omega}}_{0}{[1\ensuremath{-}\frac{4}{n(n+3)}]}^{\frac{1}{2}}$, where $n=1,3,5,\dots{}$ and ${\ensuremath{\omega}}_{0}$ is the unperturbed optical-phonon frequency. For $n=1$, ${\ensuremath{\Omega}}_{1}=0$ and this mode is a translation. For even-parity modes, the phonon frequency spectrum is determined numerically.
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