Photocatalytic Degradation of Methyl Orange over Nitrogen–Fluorine Codoped TiO<sub>2</sub> Nanobelts Prepared by Solvothermal Synthesis

Zuoli He, Wenxiu Que, Jing Chen, Xingtian Yin, Yucheng He, Jiangbo Ren

ACS Applied Materials & Interfaces · 2012 · 117 citations · 36 references

Concepts

Abstract

Anatase type nitrogen-fluorine (N-F) codoped TiO(2) nanobelts were prepared by a solvothermal method in which amorphous titania microspheres were used as the precursors. The as-prepared TiO(2) nanobelts are composed of thin narrow nanobelts and it is noted that there are large amount of wormhole-like mesopores on these narrow nanobelts. Photocatalytic activity of the N-F codoped TiO(2) nanobelts was measured by the reaction of photocatalytic degradation of methyl orange. Results indicate that the photocatalytic activity of the N-F codoped TiO(2) nanobelts is higher than that of P25, which is mainly ascribed to wormhole-like mesopores like prison, larger surface area, and enhanced absorption of light due to N-F codoping. Interestingly, it is also found that the photocatalytic activity can be further enhanced when tested in a new testing method because more photons can be captured by the nanobelts to stimulate the formation of the hole-electron pair.

References

36