Physical Review Letters · 2004 · 265 citations · 23 references
EngineeringPhysicsColloid ScienceCondensed Matter PhysicsTransport PhenomenaBrownian MotionDiffusion ProcessesOptical TweezersTime-dependent TransportBrownian Motion In SuspensionsBrownian Motion Near InterfacesColloidal SolutionsDiffusion In ColloidsDiffusive TransportParticle DiffusionParticle TransportSingle-file Diffusion
We study the diffusive behavior of colloidal particles which are confined to one-dimensional channels generated by scanning optical tweezers. At long times t, the mean-square displacement is found to scale as t(1/2), which is expected for systems where single-file diffusion occurs. In addition, we experimentally obtain the long-time, self-diffusive behavior from the short-time collective density fluctuations of the system as suggested by a recent analytical approach [Phys. Rev. Lett. 90, 180602 (2003)].
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