Ultranarrow Luminescence Lines from Single Quantum Dots

Marius Grundmann, J. Christen, N. N. Ledentsov, J. Böhrer, D. Bimberg, S.S. Ruvimov, P. Werner, Uwe Richter, U. Gösele, J. Heydenreich,

Physical Review Letters · 1995 · 738 citations · 18 references

Concepts

TL;DR

Quantum dots were fabricated by molecular beam epitaxy using a strain‑induced self‑organizing mechanism. Ultranarrow (<0.15 meV) cathodoluminescence lines from single InAs quantum dots in GaAs were observed up to 50 K, confirming δ‑function‑like electronic states, with a narrow size distribution (12 ± 1 nm) and a dense array producing an absorption peak that aligns with the luminescence maximum.

Abstract

We report ultranarrow $(&lt;0.15\mathrm{meV})$ cathodoluminescence lines originating from single InAs quantum dots in a GaAs matrix for temperatures up to 50 K, directly proving their $\ensuremath{\delta}$-function-like density of electronic states. The quantum dots have been prepared by molecular beam epitaxy utilizing a strain-induced self-organizing mechanism. A narrow dot size distribution of width $12\ifmmode\pm\else\textpm\fi{}1\mathrm{nm}$ is imaged by plan-view transmission electron microscopy. Cathodoluminescence images directly visualize individual dot positions and recombination from a single dot. A dense dot array $(\ensuremath{\sim}{10}^{11}\mathrm{dots}/{\mathrm{cm}}^{2})$ gives rise to a distinct absorption peak which almost coincides with the luminescence maximum.

References

18