Strong-Field Double Ionization through Sequential Release from Double Excitation with Subsequent Coulomb Scattering

Abstract

We perform a triple coincidence study on differential momentum distributions of strong-field double ionization of Ar atoms in linearly polarized fields (795 nm, 45 fs, 7×10(13) W/cm2). Using a three-dimensional two-electron atomic-ensemble semiclassical model including the tunneling effect for both electrons, we retrieve differential momentum distributions and achieve a good agreement with the measurement. Ionization dynamics of the correlated electrons for the side-by-side and back-to-back emission is analyzed separately. According to the semiclassical model, we find that the doubly excited states are largely populated after the laser-assisted recollision and large amounts of double ionization dominantly takes place through sequential ionization of doubly excited states at such a low laser intensity. Compared with the Coulomb-free and Coulomb-corrected sequential tunneling models, we verify that electrons can obtain an energy as large as ∼6.5U p through Coulomb scattering in the combined laser and doubly charged ionic fields.