Physical review. B, Condensed matter · 2002 · 48 citations · 14 references
Natural SciencesPhysicsCondensed Matter PhysicsOptoelectronicsQuantum MechanicsElectron-phonon InteractionsOptical Properties Of SemiconductorsOptoelectronic MaterialsQuantum ConfinementQuantum DotsQuantum OptoelectronicsEnergy RelaxationExciton-phonon CouplingExcitonsPhononsPhotoluminescenceQuantum Dot PhotophysicsStrong CouplingStrong Coupling Effects
We present the results of energy relaxation calculations for electron-hole pairs confined in a quantum dot and in strong coupling with LO phonons (excitonic polarons). We show that despite the robustness of the polaron entity, its disintegration induced by the anharmonic decay of its LO phonon component can lead to an efficient energy relaxation. We compute the time-dependent photoluminescence signals associated with the ground-state excitonic polaron as well as the photoluminescence excitation signal and the energy loss rate of an excitonic polaron in a quantum dot. Our calculations clearly evidence the existence of dot parameters where the energy relaxation is inhibited.
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Observation of Phonon Bottleneck in Quantum Dot Electronic Relaxation
Junji Urayama, Theodore B. Norris, J. Singh et al. · Physical Review Letters · 2001 · 367 citations