Coherent-population-trapping resonances in buffer-gas-filled Cs-vapor cells with push-pull optical pumping

Abstract

We report on a theoretical study and experimental characterization of coherent-population-trapping (CPT) resonances in buffer-gas-filled vapor cells with push-pull optical pumping (PPOP) on Cs ${D}_{1}$ line. We point out that the push-pull interaction scheme is identical to the so-called $\mathrm{lin}\ensuremath{\perp}\mathrm{lin}$ polarization scheme. Expressions of the relevant dark states, as well as of absorption, are reported. The experimental setup is based on the combination of a distributed feedback diode laser, a pigtailed intensity Mach-Zehnder electro-optic modulator (MZ EOM) for optical sideband generation and a Michelson-like interferometer. A microwave technique to stabilize the transfer function operating point of the MZ EOM is implemented for proper operation. A CPT resonance contrast as high as 78$%$ is reported in a cm-scale cell for the magnetic-field-insensitive clock transition. The impact of the laser intensity on the CPT-clock signal key parameters (linewidth, contrast, linewidth/contrast ratio) is reported for three different cells with various dimensions and buffer-gas contents. The potential of the PPOP technique for the development of high-performance atomic vapor-cell clocks is discussed.