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Positron annihilation in gaseous hydrogen and hydrogen-neon mixtures. II. Positronium
24
Citations
20
References
1979
Year
Chemical EngineeringPositron AnnihilationEngineeringNuclear PhysicsPhysicsAnnihilation RateNatural SciencesHigh-energy Nuclear ReactionHydrogen TransitionPositron Annihilation SpectroscopyNuclear TheoryAtomic PhysicsPartial DensitiesHydrogenChemistryQuantum ChemistryAnnihilation RatesChemical Kinetics
The annihilation rate of positrons bound in $o$-Ps atoms and the fraction of positrons which form Ps have been measured for ${\mathrm{H}}_{2}$ gas at 293, 250, and 77 K at densities in the range 5.9-429 amagat, and for ${\mathrm{H}}_{2}$-Ne gas mixtures at 77 K having ${\mathrm{H}}_{2}$ partial densities in the range 1.9-286 amagat and with Ne concentrations in the range 0.02-0.98. Large deviations from the annihilation rates expected for free $o$-Ps atoms are observed and are attributed to the formation of localized cavity states. The results obtained with ${\mathrm{H}}_{2}$-Ne mixtures strongly support $o$-Ps-induced cavity formation. Complex density and temperature dependencies are observed for the Ps fraction in ${\mathrm{H}}_{2}$, and the addition of partial densities of Ne enhances positronium formation. The annihilation of slow positrons in ${\mathrm{H}}_{2}$ is discussed in paper I of this series.
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