Journal of Applied Physics · 2012 · 31 citations · 31 references
Natural SciencesMaterials EngineeringMaterials ScienceNanotechnologyOptical MaterialsPhotonicsNanostructured SurfacesPhotonic MaterialsPlasmonic MaterialsPlasmonic NanomaterialsPlasmonicsSurface PhysicsGold NanostructuresMie ScatteringPlasmonic NanoparticlesPlasmonic NanostructuresPlasmonic SurfacesStimulated EmissionSurface Plasmonic NanostructuresSurface Plasmonic Properties
Surface plasmon (SP) amplification by stimulated emission of radiation (spaser) of the active nanoshell with three-layer silica-gold-silica structure is proposed. The properties of the spaser are numerically analyzed based on Mie theory. The results show that the nanoshell-based spaser is one order of magnitude higher than the nanosphere-based and nanoegg-based spasers in the surface plasmon amplification, but the gain threshold kthre of the silica is nearly one order of magnitude lower. In addition, the behavior of the nanoshell-based spaser depends on structural parameters that are explained by the quenching effect, plasmon hybridization theory, and dynamic photon-plasmon coupling mechanism. By optimizing the structure parameters of the layered nanoshell, an extremely high spaser enhancement over a wider operating range of wavelength tunings was obtained, both aspects having important significance in practical applications.
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