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Assessing different forms of the strong-field approximation for harmonic generation in molecules
31
Citations
15
References
2007
Year
EngineeringAcceleration FormComputational ChemistryHarmonic GenerationHarmonic SpaceNonlinear Wave PropagationBiophysicsQuantum SciencePhysicsNon-linear OpticDifferent FormsAtomic PhysicsPhysical ChemistryQuantum ChemistryStrong-field ApproximationVelocity FormNatural SciencesApplied PhysicsHigh-frequency ApproximationWave Interference
We analyse three different formulations of the strong-field approximation for high-harmonic generation in diatomic molecules, based on length, velocity and acceleration form for the recombination amplitude. We compare the predictions for the two-centre interference with those from the time-dependent Schrödinger equation. We find that the velocity form gives the closest agreement with the exact results while being the simplest from a computational point of view.
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