Magnetic properties of <i>n</i>-GaMnN thin films

G. T. Thaler, M. E. Overberg, R. M. Frazier, C. R. Abernathy, S. J. Pearton, Jong‐Soo Lee, Sungwon Lee, Y. D. Park, Z. G. Khim, J. Kim,

Applied Physics Letters · 2002 · 332 citations · 21 references

Concepts

TL;DR

GaMnN thin films were synthesized by gas‑source molecular‑beam epitaxy with Mn concentrations ranging from 3 % to 12 % at. The films exhibited no secondary phase, were n‑type, and displayed room‑temperature ferromagnetism with a Curie temperature above 320 K, with 3 % Mn showing the strongest ordering per Mn atom.

Abstract

GaMnN thin films were synthesized using gas-source molecular-beam epitaxy. Mn concentrations between 3 and 12 at. % were investigated. No evidence of second-phase formation was observed by powder x-ray diffraction or high-resolution cross section transmission electron microscopy in films with 9% or less Mn. The films were n type as determined by capacitance–voltage or Hall analysis. Magnetic characterization performed using a squid magnetometer showed evidence of ferromagnetic ordering at room temperature for all samples. In agreement with theoretical predictions, material with 3% Mn showed the highest degree of ordering per Mn atom. At 320 K, the samples show a nonzero magnetization indicating a TC above room temperature.

References

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