Publication | Open Access
Predicting the Long-Time Dynamic Heterogeneity in a Supercooled Liquid on the Basis of Short-Time Heterogeneities
295
Citations
26
References
2006
Year
Quantum LiquidLong-time Dynamic HeterogeneityEngineeringGlass-forming LiquidLiquid-liquid FlowGlass MaterialLocal Debye-waller FactorSoft MatterSimple LiquidGlass TransitionNumerical SimulationSpatial DistributionGlass-forming MixtureShort-time HeterogeneitiesPhysicsSupercritical FlowSupercooled LiquidPhase EquilibriumNatural SciencesApplied PhysicsCondensed Matter PhysicsMultiscale Modeling
We report that the local Debye-Waller factor in a simulated 2D glass-forming mixture exhibits significant spatial heterogeneities and that these short-time fluctuations provide an excellent predictor of the spatial distribution of the long-time dynamic propensities [Phys. Rev. Lett. 93, 135701 (2004)]. In contrast, the potential energy per particle of the inherent structure does not correlate well with the spatially distributed dynamics.
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