Physical Review B · 2009 · 157 citations · 59 references
Natural SciencesMaterials SciencePhysicsFluid DynamicsMechanical Behavior Of MaterialsStructural AnalysisShock ResponseShock WavesCompressionHigh-pressure Equation Of StateImpedance Data FittingLaser-driven Shock WavesShock DynamicsShock LoadingShock Wave DynamicsSystematic Errors
Laser‑driven shock loading of liquid deuterium between 45 and 220 GPa was characterized by impedance matching to an aluminum standard, with an Al impedance‑match model fitted to absolute Hugoniot data used to reduce systematic errors from the high‑pressure Al equation of state. The measurements show that deuterium compresses to η≈4.2 below 100 GPa and reaches a maximum η≈5.0 between 100 and 220 GPa—less than earlier laser‑shock results but higher than extrapolations—and reveal an abrupt compression increase near 110 GPa, in agreement with previous double‑shock data.
The compression $(\ensuremath{\eta})$ of liquid deuterium between 45 and 220 GPa under laser-driven shock loading has been measured using impedance matching to an aluminum (Al) standard. An Al impedance-match model derived from a best fit to absolute Hugoniot data has been used to quantify and minimize the systematic errors caused by uncertainties in the high-pressure Al equation of state. In deuterium below 100 GPa results show that $\ensuremath{\eta}\ensuremath{\simeq}4.2$, in agreement with previous impedance-match data from magnetically driven flyer and convergent-explosive shock wave experiments; between 100 and 220 GPa $\ensuremath{\eta}$ reaches a maximum of $\ensuremath{\sim}5.0$, which is less than the sixfold compression observed on the earliest laser-shock experiments but greater than expected from simple extrapolations of lower-pressure data. Previous laser-driven double shock results are found to be in good agreement with these single shock measurements over the entire range under study. Both sets of laser-shock data indicate that deuterium undergoes an abrupt increase in compression at around 110 GPa.
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On the Possibility of a Metallic Modification of Hydrogen
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