Giant magnetoelectric effect in nonlinear Metglas/PIN-PMN-PT multiferroic heterostructure

Abstract

In this paper, we demonstrate high converse magnetoelectric (ME) coupling in a Metglas/Pb(In1/2Nb1/2)O3-Pb(Mg1/3Nb2/3)O3-PbTiO3 (PIN-PMN-PT) laminated ME composite by exploiting stress and field induced reversible ferroelectric-ferroelectric phase transitions in a relaxor ferroelectric single crystal. The approach exploits large transformational strain induced by low applied electric field in a PIN-PMN-PT crystal that was mechanically stressed close to a rhombohedral to orthorhombic phase transformation. The ME coefficient was enhanced by an order of magnitude as compared to the linear piezoelectric regime, with a maximum value of 1.3 × 10−7 s m−1 in non-resonant mode. This phenomenon can thus be exploited to provide improvements in the development of ME devices and magnetic sensors.