High-field terahertz response of graphene

M. J. Paul, You-Chia Chang, Z. Thompson, Andrew D. Stickel, Jenna L. Wardini, Ethan D. Minot, B. Hou, J. Nees, Theodore B. Norris, Yun-Shik Lee

New Journal of Physics · 2013 · 85 citations · 43 references

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Abstract

doi:10.1088/1367-2630/15/8/085019 Abstract. We investigate the response of multi-layer epitaxial graphene and chemical vapor deposition (CVD)-grown single-layer graphene to strong terahertz (THz) fields. Contrary to theoretical predictions of strong nonlinear response, the transmitted fields exhibit no harmonic generation, indicating that the nonlinear response is limited by fast electron thermalization due to carrier–carrier scattering. The fast electron heating gives rise to large THz transmission enhancement (>15%) in single-layer CVD graphene at high THz fields (ETHz> 10 kV cm−1). The nonlinear effects exhibit non-Drude behavior in the THz conductivity, where THz fields induce extreme non-equilibrium electron distributions. 4 Author to whom any correspondence should be addressed. Content from this work may be used under the terms of the Creative Commons Attribution 3.0 licence. Any further distribution of this work must maintain attribution to the author(s) and the title of the work, journal citation and DOI.

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