Dalton Transactions · 2012 · 46 citations · 41 references
Natural SciencesChemistryOrganic ChemistryOrganometallic ChemistryStructure-activity RelationshipsCoordination ChemistrySupramolecular MaterialsAqueous-phase SynthesisComplexation ChemistryHydroformylationSchiff Base Catalysis
Water-soluble dendritic ligands based on tris-2-(5-sulfonato salicylaldimine ethyl)amine (5) and DAB-(5-sulfonato salicylaldimine) (6) (DAB = diaminobutane) were synthesized by means of Schiff base condensation and sulfonation reactions. These dendritic ligands were fully characterized by (1)H NMR, (13)C NMR and FT-IR spectroscopy, elemental analysis and mass spectrometry. Dendritic ligands (5 and 6) in combination with [RhCl(COD)](2) (COD = 1,5-cyclooctadiene) were evaluated in aqueous biphasic hydroformylation of 1-octene. New water-soluble mononuclear 5-sulfonato propylsalicylaldimine Rh(i) complexes (7 and 8) were synthesized and characterized using (1)H NMR, (13)C NMR and FT-IR spectroscopy, elemental analysis as well as mass spectrometry. These complexes were applied as catalyst precursors in aqueous biphasic hydroformylation reactions. All the catalyst precursors were active in the hydroformylation of 1-octene under the investigated conditions. Optimal conditions were realized at 75 °C (40 bars), where the best selectivity for aldehydes was noticed. Catalyst recycling was achieved up to 5 times with minimal loss in conversion and consistent chemoselectivities and regioselectivities. Less Rh leaching was observed in the dendritic systems (5 and 6)/[RhCl(COD)](2) as compared to mononuclear catalyst precursors (7 and 8) as determined by inductively coupled plasma-mass spectrometry (ICP-MS).
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Progress in hydroformylation and carbonylation
Matthias Beller, B. Cornils, C.‐D. Frohning et al. · Journal of Molecular Catalysis A Chemical · 1995 · 872 citations