Physical Review Letters · 2004 · 392 citations · 15 references
Natural SciencesPhysicsComputational Fluid DynamicsCondensed Matter PhysicsFluid DynamicsSolid-liquid InterfacesStates Of MatterDynamic HeterogeneityHeterogeneityParticle DynamicsParticle-liquid InteractionsSpatial Distribution PatternsStatistical Mechanics Of LiquidsSupercritical Fluid Behavior
The particle dynamics in a liquid exhibits a transient spatial distribution of dynamic heterogeneities. The relationship between this kinetic structure and the underlying particle configuration remains an outstanding problem. In this Letter, we present a general simulation technique for identifying the features of the dynamic heterogeneity which arise due to a specific configuration, as distinct from the random spatial variation due to the intermittent particle dynamics.
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What Do We Learn from the Local Geometry of Glass-Forming Liquids?
Francis W. Starr, Srikanth Sastry, Jack F. Douglas et al. · Physical Review Letters · 2002 · 297 citations · Full text