The role of finite magnetic clusters in Au-Fe alloys near the percolation concentration

TLDR

Au‑Fe alloys have been investigated via magnetic measurements across the composition range where ferromagnetism transitions from spin‑glass behavior. The study identifies a percolation threshold at 15.5 % Fe, finds that between 15.5 % and ~28 % Fe finite magnetic clusters coexist with the infinite cluster and freeze at a characteristic temperature, and reports magnetic resonance above ~13 % Fe with linewidth temperature dependence matching the magnetization behavior.

Abstract

Abstract Au-Fe alloys have been studied by magnetic measurements of various types in the composition range where ferromagnetism evolves from spin-glass character. The percolation limit identified from the results and other data is 15.5 + 0.3 at.% Fe. Between this composition and ∼28% Fe, finite clusters co-exist in significant concentrations with the infinite cluster, and a fairly well-defined temperature observed in the magnetic properties is ascribed to a freezing of these clusters that parallels that of finite clusters in the pre-percolation alloys. Magnetic resonance is observed in alloys with more than about 13% Fe (i.e. in alloys containing large nearest-neighbour clusters) and the temperature dependence of the linewidth correlates with the interpretation given of the magnetization data.