Publication | Closed Access
Oscillatory Clusters in the Periodically Illuminated, Spatially Extended Belousov-Zhabotinsky Reaction
95
Citations
15
References
2001
Year
Optical MaterialsEngineeringLocalized Excited StateAutonomous Bz SystemNegative Global FeedbackComputational ChemistryChemistryElectronic Excited StateCluster-cluster TransitionsOptical PropertiesPhotophysical PropertyCluster ScienceOscillatory ClustersPhysicsPhotochemistryMechanistic PhotochemistryAtomic PhysicsPhysical ChemistryQuantum ChemistryPhotochromismExcited State PropertyNatural SciencesApplied Physics
Cluster-cluster transitions in the periodically illuminated photosensitive Belousov-Zhabotinsky (BZ) reaction-diffusion system exhibit the same scenario as in the autonomous BZ system with negative global feedback: two-phase clusters <--> three-phase clusters <--> irregular clusters <--> localized clusters. Transitions induced by changing the dark ( TD) or light ( TL) phases of the periodic external square wave illumination are dependent not only on the frequency of illumination at constant TD/TL, but also on the ratio TD/TL at constant frequency (when TD+TL = const).
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