Geophysical Research Letters · 2004 · 223 citations · 14 references
Natural SciencesEarth SciencesEnvironmental SciencesAtmospheric ChemistryAtmospheric ScienceClimatologyAir Pollution SourcesBiogeochemical Cycle ModelingCarbon CycleCarbon Emissions MeasurementCarbon MonoxideTropospheric ChemistryCarbon Monoxide Atmospheric ChemistryCarbon Monoxide BudgetCarbon Monoxide MeasurementCarbon Monoxide ModelingCarbon Monoxide SourcesEmission Inventory ModelingInverse Modeling For Emission EstimationSatellite-based Emissions Estimation
This paper presents results of the inverse modeling of carbon monoxide surface sources on a monthly and regional basis using the MOPITT (Measurement Of the Pollution In The Troposphere) CO retrievals. The targeted time period is from April 2000 to March 2001. A sequential and time‐dependent inversion scheme is implemented to correct an a priori set of monthly mean CO sources. The a posteriori estimates for the total anthropogenic (fossil fuel + biofuel + biomass burning) surface sources of CO in TgCO/yr are 509 in Asia, 267 in Africa, 140 in North America, 90 in Europe and 84 in Central and South America. Inverting on a monthly scale allows one to assess a corrected seasonality specific to each source type and each region. Forward CTM simulations with the a posteriori emissions show a substantial improvement of the agreement between modeled CO and independent in situ observations.
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