Publication | Closed Access
Observation of Front Bifurcations in Controlled Geometries: From One to Two Dimensions
65
Citations
19
References
1995
Year
EngineeringControlled GeometriesConcentration WavesChemistryStabilityCatalytic ReactionFront BifurcationsPhysicsChaos TheoryChemisorptionBifurcation TheorySurface ChemistryNatural SciencesSurface AnalysisSurface ScienceApplied PhysicsMechanical SystemsReaction ProcessChemical KineticsSurface ReactivityNonlinear Oscillation
The introduction of microstructures in the form of quasi-one-dimensional channels on a Pt(100) surface allows the detection of front bifurcations for concentration waves from adsorbed O and CO species accompanying their catalytic reaction. At the exits of these channels into larger circular domains, the fronts can be reflected depending on the width of the channels and the external parameters. These findings are reproduced within a reaction-diffusion model.
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