Coexistence of reentrant-spin-glass and ferromagnetic martensitic phases in the Mn2Ni1.6Sn0.4 Heusler alloy

Abstract

A giant exchange bias field of up to 1170 Oe was observed in the Mn2Ni1.6Sn0.4 Heusler alloy. A reentrant spin glass phase and a ferromagnetic martensitic phase coexist below the blocking temperature as confirmed by dc magnetization and ac susceptibility measurements. Exchange bias in Mn2Ni1.6Sn0.4 is thought to originate from the interface exchange interaction between the reentrant spin glass phase and the ferromagnetic martensitic phase. X-ray diffraction and selected area electron diffraction results demonstrate that excess Mn atoms occupy Ni and Sn sites randomly. In this way, Mn-Mn clusters are formed and constitute the reentrant-spin-glass phase.