Cooperative effects on multiphoton ionization and third-harmonic generation in the region near three-photon resonance

Abstract

Three-photon resonance enhancement of third-harmonic generation and multiphoton ionization is treated for a slab geometry configuration. Striking pressure effects which become important at concentrations $n\ensuremath{\gtrsim}{10}^{12}$ ${/\mathrm{c}\mathrm{m}}^{3}$ for narrow-bandwidth short-pulse lasers are predicted for both the third-harmonic signal and the multiphoton ionization. For example, part of the third-harmonic signal exists the slab simultaneously with the laser pulse while another part is time delayed for small detunings from resonance. At intermediate detuning from the three-photon resonance the two parts can interfere. Multiphoton ionization yields near three-photon resonance are strongly suppressed under certain conditions, and peaks may occur for proper detunings on both sides of the three-photon resonance. A detailed experimental verification is suggested for Xe.