Influence of the dynamic Stark effect on photoelectron angular distributions in multiphoton ionization

Abstract

The influence of the dynamic Stark effect on photoelectron angular distributions for two-photon-resonant three-photon ionization of sodium by way of the $4^{2}D$ fine-structure components has been investigated. Owing to the dynamic Stark shift of the atomic transition frequency, the angular distributions expected at low laser intensities were modified as different transitions were intensity tuned into and out of resonance with the laser frequency. The distributions are in good qualitative agreement with theory.