Dipole Blockade at Förster Resonances in High Resolution Laser Excitation of Rydberg States of Cesium Atoms

Abstract

High resolution laser excitation of np Rydberg states of cesium atoms shows a dipole blockade at Förster resonances corresponding to the resonant dipole-dipole energy transfer of the np+np --> ns+(n+1)s reaction. The dipole-dipole interaction can be tuned on and off by the Stark effect, and such a process, observed for relatively low n(25-41), is promising for quantum gate devices. Both Penning ionization and saturation in the laser excitation can limit the range of observation of the dipole blockade.