Journal of Physics D Applied Physics · 2012 · 36 citations · 22 references
EngineeringSupercritical Fluid ChromatographyInitiation MechanismGlow DischargePressurized Carbon DioxideInitiation ProcessSupercritical FlowPulse PowerMultiphase FlowPositive StreamerGas Discharge PlasmaBurst Primary StreamerSupercritical Co2
Abstract In this work, the initiation process of an electrical discharge in pressurized carbon dioxide up to the liquid and supercritical phases was investigated using Schlieren and photomultiplier techniques. A pulsed positive voltage with a rise time of about 40 ns and half-width of 150 ns was applied to a point-to-plane gap. The experimental results showed that the discharge started with a primary streamer consisting of a burst primary streamer and a successive primary streamer, and a back discharge followed them. It was predicted from an analysis of the experimental results that the initiation criterion of a burst primary streamer was electron multiplication on the order of 10 8 independent of the medium conditions. That is, a direct ionization process without bubble formation is supported as an initiation mechanism of nanosecond positive discharges in pressurized carbon dioxide. The medium state in the burst primary streamer channel was a gas or pseudo-gas of 50–200 kg m −3 density.
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