Physical Review A · 2011 · 46 citations · 62 references
Natural SciencesChemistryPhysicsChemical KineticsMolecular PhysicsPhysical ChemistryCluster ChemistryCollision TheoryIonization ProcessesMolecular CollisionsReaction DynamicsCoulomb ExplosionElectron Impact CollisionsFragmentation PathwaysHigh-energy Collision DynamicsIon-ion CollisionsIonizationMolecular ClustersMolecular Collision Dynamics
We report on an experimental study of the ionization and fragmentation of clusters of $k$ polycyclic aromatic hydrocarbon (PAH) molecules using anthracene, C${}_{14}$H${}_{10}$, or coronene, C${}_{24}$H${}_{12}$. These PAH clusters are moderately charged and strongly heated in small impact parameter collisions with 22.5-keV He${}^{2+}$ ions, after which they mostly decay in long monomer evaporation sequences with singly charged and comparatively cold monomers as dominating end products. We describe a simple cluster evaporation model and estimate the number of PAH molecules in the clusters that have to be hit by He${}^{2+}$ projectiles for such complete cluster evaporations to occur. Highly charged and initially cold clusters are efficiently formed in collisions with 360-keV Xe${}^{20+}$ ions, leading to cluster Coulomb explosions and several hot charged fragments, which again predominantly yield singly charged, but much hotter, monomer ions than the He${}^{2+}$ collisions. We present a simple formula, based on density-functional-theory calculations, for the ionization energy sequences as functions of coronene cluster size, rationalized in terms of the classic electrostatic expression for the ionization of a charged conducting object. Our analysis indicates that multiple electron removal by highly charged ions from a cluster of PAH molecules rapidly may become more important than single ionization as the cluster size $k$ increases and that this is the main reason for the unexpectedly strong heating in these types of collisions.
62
Yan Zhao, Donald G. Truhlar · Theoretical Chemistry Accounts · 2007 · 30K citations · Full text
Natural Sciences, Chemistry, Physics +17
Reaction mechanism of soot formation in flames
Michael Frenklach · Physical Chemistry Chemical Physics · 2002 · 1.5K citations