Physical Review Letters · 2012 · 93 citations · 28 references
Natural SciencesPhysicsCondensed Matter PhysicsOptical MaterialsOpticsLaser PhysicsNonlinear OpticsOptical Properties Of SolidsRefractive IndexThin Film Optical PropertiesUltrafast OpticsAnomalous DispersionGroup IndexGroup Refractive IndexHeterodyne InterferometryOptical Pulse PropagationPhase Shift MeasurementsPulse PropagationRefraction
We present an experimental measurement of the refractive index of high density Rb vapor in a gaseous atomic nanolayer. We use heterodyne interferometry to measure the relative phase shift between two copropagating laser beams as a function of the laser detuning and infer a peak index $n=1.26\ifmmode\pm\else\textpm\fi{}0.02$, close to the theoretical maximum of 1.31. The large index has a concomitant large index gradient creating a region with steep anomalous dispersion where a subnanosecond optical pulse is advanced by $>100\text{ }\text{ }\mathrm{ps}$ over a propagation distance of 390 nm, corresponding to a group index ${n}_{g}=\ensuremath{-}(1.0\ifmmode\pm\else\textpm\fi{}0.1)\ifmmode\times\else\texttimes\fi{}{10}^{5}$, the largest negative group index measured to date.
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