Energy Procedia · 2011 · 46 citations · 5 references
EngineeringChemical EngineeringEnvironmental EngineeringProcess DynamicsProcess Systems EngineeringReaction EngineeringCarbon CaptureCarbon Dioxide RemovalCarbon SequestrationReaction Process DesignReactor ModelingTransient AnalysisCarbon Dioxide CaptureCarbon Dioxide Removal ModelingExperimental Results InterpretationOperational ConditionsParametric Sensitivity AnalysisReaction Rate Constant EstimationSensitivityTransient State Analysis
Considerable effort on research in CO2 capture technologies has been directed towards steady state systems while less seems to have been done for the same systems in transient state. This work presents a dynamic model for CO2 absorption using aqueous mono-ethanolamine (MEA). Validation against experimental results both obtained at steady state and dynamic conditions is included. A parametric sensitivity study of the underlying model equations is carried out based alternative parameter correlations for the reaction rate constant. It is concluded that validated results for one specific pilot plant don’t necessarily apply to other plants of different sizes under other operational conditions. Furthermore, a parametric sensitivity study for the other parameters as well as for the rest of the CO2 capture process is also warranted.
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Karl Anders Hoff, Olav Juliussen, Olav Falk-Pedersen et al. · Industrial & Engineering Chemistry Research · 2004 · 142 citations · Full text